The below little code snippet will help you to do that by using DayRender event of Calendar control.
.ASPX
<asp:Calendar ID="Calendar1" runat="server" ondayrender="Calendar1_DayRender"> </asp:Calendar>
CodeBehind
protected void Calendar1_DayRender(object sender, DayRenderEventArgs e)
{
if (e.Day.Date.DayOfWeek == DayOfWeek.Monday)
{
e.Day.IsSelectable = false;
}
}
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